Frank Welker

Azrael (voice)

Hank Azaria

Gargamel

Neil Patrick Harris

Patrick Winslow

Sofía Vergara

Odile Anjelou

Jayma Mays

Grace Winslow

Jonathan Winters

Papa Smurf (voice)

Katy Perry

Smurfette (voice)

Anton Yelchin

Clumsy Smurf (voice)

Tim Gunn

Henri

Madison McKinley

Model

Meg Phillips

Model

Mahadeo Shivraj

Cabbie

Julie Chang

Newscaster

Mark Doherty

Bluetooth Businessman

Minglie Chen

Young Woman

Sean Kenin

Guy in Plaid Shirt

Victor Pagan

Bum

Adria Baratta

Anjelou Employee

Paula Pizzi

Odile's Mother

Andrew Sellon

Waiter

Julianna Rigoglioso

Little Sister

Daria Rae Figlo

Blonde Sister

Bradley Gosnell

Toy Salesperson

Heidi Armbruster

Toy Store Parent

Raja Gosnell

Director

Ben Haber

Executive Producer

Paul Neesan

Executive Producer

Ezra Swerdlow

Executive Producer